CHAPTER 16 final.docx

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AMENDMENT 0005: Reactor Recovery Services Federal contract opportunity
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1333ND25RNB610012
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Department of Commerce National Institute of Standards and Technology

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This file is Chapter 16 from what appears to be a technical manual or safety analysis report for the National Bureau of Standards Reactor (NBSR), focusing on license considerations and reactor component inspections. The chapter details inspection results of the reactor vessel's interior and exterior components, conducted in 2000 and 2002, which found no significant flaws or defects that would affect operational integrity. It includes specific data on mechanical testing of aluminum alloy components and their response to radiation exposure over time.

The chapter provides technical specifications for reactor vessel embrittlement analysis, particularly regarding the aluminum alloys 5052 and 6061 used in construction, with detailed test results showing changes in tensile strength, elongation, and impact energy after radiation exposure. The document confirms that the NBSR is not used for medical purposes and includes calculations projecting that the most heavily irradiated positions will accumulate less than 2x10^23 n-cm^-2-s^-1 thermal neutron fluence by 2024, maintaining sufficient ductility for safe operation. A table of mechanical test results comparing irradiated versus unirradiated specimens is included, showing specific measurements for tensile strength, elongation, impact energy, and fracture toughness.

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CHAPTER 16 – TABLE OF CONTENTS

16OTHER LICENSE CONSIDERATIONS1
16.1Prior Use Of Reactor Components1
16.1.1Reactor Vessel and Core Components1
16.1.1.1Reactor Vessel Interior Inspection1
16.1.1.2Reactor Vessel Exterior Inspection2
16.1.1.3Reactor Vessel Embrittlement2
16.2Medical Use of Non-Power Reactors3
16.3References3

List of Tables

Table 16.1: NBSR Reactor Vessel Mechanical Test Results 4

Chapter 16 – Record of Revisions

Revision
Date
ECN
Description
Changed By
Reviewed By
Approved By
7
xx/xx/15
Update of Chapter 16, including cavity purge system content.
T. Myers

16 OTHER LICENSE CONSIDERATIONS Comment by Myers, Thomas J.: Only aging issues. Replacement of important (Chapter 13) components, radiation damage, etc. Is source storage/byproduct material something that should be included? That is, coordination of two licenses, NIST materials and NIST reactor. ROE question. Answered 12/2/15. No changes. DONE.

This Chapter discusses the prior use of components in the NBSR and documents that the reactor has only been used solely for non-medical research.

16.1 Prior Use Of Reactor Components

The NBSR initiated neutron research in 1969. Chapter 1.8 discusses the facility history and major modifications made to the facility. With the exceptions of the modifications described, all the systems, structures, and components installed and operated in the past will continue to be used in the NBSR. Design and operating limits, the potential for age-related degradation, inspections to assess aging, and a discussion on the suitability for continued use have been included for specific systems, structures, and components in the appropriate chapter herein (Chapter 3 Systems, Structures, and Components; Chapter 4 Reactor including fuel, control elements, and Chapter 6 Reactor Coolant System). Additional information on the continued acceptability of use of the reactor vessel and major core components is discussed in this chapter.

16.1.1 Reactor Vessel and Core Components

Opportunities to inspect the NBSR reactor vessel are limited since the core must be offloaded to reduce interior radiation levels and allow better visibility of the vessel walls. Two types of inspections are possible: a visual inspection using binoculars when the refueling head is removed from the top of the vessel and an inspection using remote imaging equipment. In preparation for continuing facility operation, a visual inspection (using binoculars) was performed in February 2000. No flaws or unusual discolorations were observed. This type of inspection will be repeated only if the refueling head is removed from the vessel, not a frequent occurrence.

Another inspection using remote imaging equipment was performed in January 2002, which included a detailed inspection of the vessel interior. A visual record of this inspection was recorded using a radiation hardened, 2.75" diameter, 10X zoom, closed circuit video camera. This inspection was performed with the reactor vessel fully defueled, but still filled with heavy water. The inspection is stored on a DVD to provide a permanent record. The exterior of the vessel and the interior of the thermal shield were also examined during the same period, and the results recorded on the same DVD. The results of this inspection are summarized below. The inspection of the vessel interior will be repeated at an appropriate time, when the core is offloaded, estimated within the next six to eight years.

16.1.1.1 Reactor Vessel Interior Inspection

The specific areas remotely examined were all or part of the tip welds for beam ports, through tubes, the cold source, and pneumatic sample thimbles; vessel penetration welds for beam ports, through tubes, the cold source, pneumatic sample thimbles, the outer plenum, outlet pipes, the dump line, and the dry transfer pipe; and vessel fabrication welds. Sections of the upper and lower grid plates, the hold-up pan, the emergency cooling system distribution pan on the upper grid, accessible vertical thimbles, and structural members for different internal components were also inspected.

The inspection revealed no flaws that indicated a decrease in the integrity of the welds. The tip welds were in excellent condition. The other items examined also appeared to have no defects that would affect their design function.

16.1.1.2 Reactor Vessel Exterior Inspection

The vertical portion of the exterior of the vessel may only be seen via a one inch (2.54 cm) gap between the thermal shield and the reactor vessel. The bottom of the reactor vessel is in an area bounded by the vessel, the thermal shield, and the one inch gap. During a cryostat maintenance activity, access to the gap was gained via the biological shield penetration for the Cold Source cryostat. The camera was inserted through the gap to the area containing the bottom of the vessel. The examination of the reactor vessel wall, the dry transfer pipe, the outlet piping, and the outer plenum did not uncover any material condition that could lead to a failure. The thermal shield within the inspection area was also found in good condition.

16.1.1.3 Reactor Vessel Embrittlement

The NBSR vessel is fabricated from aluminum alloys 5052 and 6061, which have been extensively studied in radiation fields. As part of the Advanced Neutron Source Project at Oak Ridge National Laboratory (ORNL), heavily irradiated (4.2x1023 thermal, 2.0x1022 fast neutrons/cm2) samples of the 6061-T6 alloy were obtained from a control rod drive follower tube used in the High Flux Beam Reactor (HFBR) at Brookhaven National Laboratory (BNL). These samples were cut into proper shapes for mechanical testing (e.g., tensile, Charpy impact, and metallographic examination) at ORNL. The results are presented in (Weeks, et al., 1993) and are summarized in Table 16.1. The authors were able to correlate their new results with all prior measurements by noting that the relevant parameters were total thermal neutron fluence and the ratio of thermal to fast fluence. Thus, the data can be assumed to be typical of results for the conditions specified above i.e. >4x1023 n-cm-2-s-1 thermal neutron fluence, and a thermal to fast fluence ratio of 20.

The most heavily irradiated portions of the NBSR vessel are the tips of the beam tubes, and the total irradiation of these components has been calculated (Rowe and Williams, 2002) using the models described in Chapter 4. The salient result is that the most heavily irradiated positions will conservatively (no extended shutdowns are included in the calculations) have accumulated less than 2x1023 n-cm-2-s-1 thermal neutron fluence by 2024. The calculations also showed that the ratio of thermal to fast fluxes ranged from 17 to 21, very analogous to those of the samples tested. Thus, the data above are a conservative estimate of the condition of the beam tube tips in the NBSR at the end-of-license. As can be seen from the irradiation data, the ductility, while reduced, retains approximately 70% of the original value, although the Charpy energy has dropped by over a factor of 6. Thus, the tips remain a ductile material, with reduced impact strength and toughness. The primary effects of the changes in properties will be reduced resistance to crack propagation under tensile stress, and reduced resistance to sudden pressure applications and impacts.

Within the NBSR, the beam tips are never under significant tensile stress. The beam tube penetrations are filled with CO2 at approximately 2 inches of water pressure (0.005 atmospheres). The cavity volume which includes the beam tips is not air tight and it is impossible to pressurize that volume with the available CO2 supply. The CO2 supply system to the cavity is protected from over-pressure by two relief valves and by a gasholder which provides a large expansion volume. No experimental systems are inside the beam tips, which are closed at the thermal shield with an aluminum window fastened to the shield (except for the cold sources, which have vessels designed to be much stronger than the vessel). Therefore, tensile stress is not an issue. The surrounding D2O does exert a compressive force (due to the static head as there is no coolant over-pressure), which causes a compressive stress, but this stress will not create cracks that can propagate quickly. The vessel is entirely closed with shielding and therefore, there can be no impacts against the beam tube tips with the shielding in place, e.g. during reactor operation.

From these considerations, it is concluded that the change in ductility of the vessel creates no hazard to continued operation of the NBSR.

16.2 Medical Use of Non-Power Reactors

The NBSR is not used for medical purposes.

16.3 References

Weeks, J. R., Czajkowski C. J., and Farrell, K. (1993). Effects of High Thermal Neutron Fluences on Type 6061 Aluminum, in Effects of Radiation on Materials: 16th International Symposium, ASTM STP 1175, A. S. Kumar, D. S. Gelles, R. K. Nanstad, and E. A. Little, Eds., American Society for Testing and Materials: Philadelphia.

Rowe, J.M. and Williams, R.E. to Weiss, Seymour (2002). Memorandum, April 4, 2002, Reactor Vessel.

Table 16.1: NBSR Reactor Vessel Mechanical Test Results

Irradiated Specimens
Unirradiated Specimens
Ultimate Tensile Strength (un-notched bar) MPa
682 10

330 4

Ultimate Tensile Strength (notched bar) MPa
200
316 27
% elongation
7.2 0.75
10.3 0.5
Charpy Impact Energy Joules
0.34 0.03
2.21 0.26
Fracture Toughness KIc (derived) (MPa m1/2)
8.7 0.8
21.75

16-4

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